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Winter Soldier - I'm Not the One by reggievass
and on tumblr here.

♥  DEPLOY / OFFLINE  ♥

Awesome Bucky/Natasha multi-source backstory vid. This impresses me so much. (Also, The Matrix isn't listed as a source, but I swear that's a Trinity scene with Scarlett's face. It's from The Perfect Score apparently. *adds to list*)